Донорно-акцепторные молекулы

При возбуждении карбазольного хромофора возбужденные состояния с карбазола мигрируют до акцепторных молекул. Последние взаимодействуют друг с другом с переходом, путем внутренней конверсии во второе возбужденное состояние с переносом заряда. При освещении в области 470 нм непосредственно возбуждается это состояние комплекса. По данным фотопроводимости рассчитана спектральная зависимость квантового выхода ионных пар в системе ПВК – тетрацианбензол. В области максимума полосы КПЗ квантовый выход, достигает значения 0,8. При более низких энергиях возбуждения квантовый выход уменьшается, что коррелирует с результатами по флуоресценции, и ее тушению. Это служит дополнительным подтверждением того, что образование, ионной пары идет из второго возбужденного состояния КПЗ.
Изучались фотоэлектрические свойства комплексов ПВК с тетрацианхинондиметаном. Было показано, что уже при небольшом содержании допанта (несколько процентов) образуется комплекс с почти панхроматической чувствительностью в видимой области спектра. Максимум фото чувствительности КПЗ расположен у 620-650 нм. Максимальная фото чувствительность достигалась при массовом соотношении ПВК и допанта 25: 1. Механизм генерации носителей интерпретируется как облегченная электрическим полем диссоциация эксиплексов и взаимодействие экситонов с захваченными на ловушках зарядами. Эффективность фото генерации зависит от напряженности поля и может быть описана в рамках модели Френкеля – Пула или Онзагера.
В части рекомбинационных процессов для КПЗ ПВК – ТНФ в соотношении 1 :1 при импульсном возбуждении рубиновым лазером было показано выполнение простой теории рекомбинации, предложенной Ланжевеном.

 

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