Линейная зависимость фото чувствительности ПВК

В спектре электро поглощения видны две полосы переноса заряда. Электро поглощение интерпретировали как энергетический сдвиг молекулярных состояний, вызванный полем, в рамках эффекта Штарка, при котором интенсивность электро поглощения квадратично зависит от напряженности электрического поля. Такая зависимость действительно была установлена. Было также показано изменение молекулярного дипольного момента и поляризации КПЗ при фото возбуждении. Перенос заряда в основном происходил только при фото возбуждении. С увеличением концентрации ТНФ концентрация молекул комплекса возрастает, стремясь к насыщению при соотношении ПВК: ТНФ 0,4:1.
При поглощении света между ПВК и ТНФ наблюдается перенос заряда по схеме Б А -> 0+А. Процесс генерации носителей может быть разделен на два этапа. Образующееся после поглощения света авто ионизирующееся состояние может ионизоваться или дезактивировать в основное состояние.
Фото генерацию носителей заряда в карбазол содержащих полимерах широко исследовали в рамках теории Онзагера, как правило, с применением электрофотографической методики. Экспериментальные и теоретические данные для квантового выхода носителей комплекса ТНФ – ПВК с соотношением компонентов 0,06: 1. Теория и эксперимент дают хорошее согласие для температур от 5 до 50°С и области напряженности полей выше 7 10» В см-1, если принять начальное расстояние разделения пары г0 =2,5 нм, а начальный квантовый выход Ф0 =0,23.

 

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