Существование короткоживущих ион-радикальных пар

Из зависимости эффективности фото генерации от напряженности электрического поля для различных длин волн в предположении одинакового начального квантового выхода следует, что величина длины термализации г0 составляет 3,0, 2,8 и 2,6 нм для третьего, второго и первого возбужденных состояний соответственно. Для различных длин термализации зависимости относительной квантовой эффективности от температуры существенно различаются. При постоянном г0 влияние температуры на выход носителей при малых напряженностях поля значительно сильнее, чем при больших. Это связано с тем, что вероятность диссоциации пары определяется напряженностью электрического поля и диффузией. Поскольку подвижность носителей и коэффициент диффузии имеют активационный характер, повышение температуры способствует процессу разделения зарядов, что уменьшает относительный вклад, вносимый в этот процесс электрическим полем. Повышение температуры приводит к возрастанию квантового выхода фото-генерации, но, по-видимому, не изменяет длину термализации. Данные эксперимента хорошо коррелируют с расчетными при условии, что с ростом температуры увеличивается начальный квантовый выход Ф0, а длина термализации остается постоянной. Начальный квантовый выход Ф0 имеет термическую энергию активации 0,05 эВ. Зависимость квантовой эффективности от температуры при различных напряженностях электрического поля также подтверждает совпадение теории Онзагера и эксперимента в пользу предположения о независимости г0 от температуры

 

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